Tuning coherent-phonon heat transport in LaCoO3/SrTiO3 Superlattices
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Title: | Tuning coherent-phonon heat transport in LaCoO3/SrTiO3 Superlattices |
Author: | Rivadulla Fernández, José Francisco Bugallo Ferrón, David Langenberg Pérez, Eric Carbo-Argibay, Enrique Varela Domínguez, Noa Otero Fumega, Adolfo Pardo Castro, Víctor Lucas del Pozo, Irene Morellón Alquézar, Luis Alberto |
Affiliation: | Universidade de Santiago de Compostela. Centro de Investigación en Química Biolóxica e Materiais Moleculares Universidade de Santiago de Compostela. Departamento de Física Aplicada Universidade de Santiago de Compostela. Departamento de Química Física |
Subject: | Interfaces | Lattices | Phonons | Thermal conductivity | Thickness | |
Date of Issue: | 2021 |
Publisher: | ACS Publications |
Citation: | J. Phys. Chem. Lett. 2021, 12, 11878−11885. https://doi.org/10.1021/acs.jpclett.1c03418 |
Abstract: | Accessing the regime of coherent phonon propagation in nanostructures opens enormous possibilities to control the thermal conductivity in energy harvesting devices, phononic circuits, etc. In this paper we show that coherent phonons contribute substantially to the thermal conductivity of LaCoO3/SrTiO3 oxide superlattices, up to room temperature. We show that their contribution can be tuned through small variations of the superlattice periodicity, without changing the total superlattice thickness. Using this strategy, we tuned the thermal conductivity by 20% at room temperature. We also discuss the role of interface mixing and epitaxial relaxation as an extrinsic, material dependent key parameter for understanding the thermal conductivity of oxide superlattices |
Publisher version: | https://doi.org/10.1021/acs.jpclett.1c03418 |
URI: | http://hdl.handle.net/10347/29025 |
DOI: | 10.1021/acs.jpclett.1c03418 |
ISSN: | 1948-7185 |
Rights: | © The Author(s) 2021. This article is licensed under a Creative Commons Attribution 4.0 International License (http://creativecommons.org/licenses/by/4.0/) |
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